Holographic generation of highly twisted electron beams

Free electrons can possess an intrinsic orbital angular momentum, similar to those in an electron cloud, upon free-space propagation. The wave front corresponding to the electron's wave function forms a helical structure with a number of twists given by the angular speed. Beams with a high number of twists are of particular interest because they carry a high magnetic moment about the propagation axis. Among several different techniques, electron holography seems to be a promising approach to shape a conventional electron beam into a helical form with large values of angular momentum. Here, we propose and manufacture a nanofabricated phase hologram for generating a beam of this kind with an orbital angular momentum up to 200h. Based on a novel technique the value of orbital angular momentum of the generated beam is measured and then compared with simulations. Our work, apart from the technological achievements, may lead to a way of generating electron beams with a high quanta of magnetic moment along the propagation direction and, thus, may be used in the study of the magnetic properties of materials and for manipulating nanoparticles.