Crossover between magnetism and superconductivity in LaFeAsO with low H-doping level

By a systematic study of the hydrogen-doped LaFeAsO system by means of dc resistivity, dc magnetometry, and muon-spin spectroscopy we addressed the question of universality of the phase diagram of rare-earth-1111 pnictides. In many respects, the behaviour of LaFeAsO1−xHxresembles that of its widely studied F-doped counterpart, with H− realizing a similar (or better) electron-doping in the LaO planes. In a x = 0.01 sample we found a long-range SDW order with TN = 118 K, while at x = 0.05 the SDW establishes only at 30 K and, below Tc = 10 K, it coexists at a nanoscopic scale with bulk superconductivity. Unlike the abrupt M-SC transition found in the parent La-1111 compound, the presence a crossover region makes the H-doped system qualitatively similar to other Sm-, Ce-, or Nd-1111 families.